24–28 Jul 2023
MPI-FKF
Europe/Berlin timezone

Establishing Coherent Momentum-Space Electronic States in Locally Ordered Materials

24 Jul 2023, 16:45
2h 45m
2D5 (MPI-FKF)

2D5

MPI-FKF

Contributed Poster Poster Session

Speaker

Dr Quentin Marsal (Uppsala Universitet)

Description

Many current and future quantum technologies rely on amorphous materials, where translational symmetry is broken, but short-range order with well-defined structural length scales persists (1). This brings forward the fundamental question whether long range order is a necessary condition to establish coherence and structured momentum-dependent electronic state, and how to characterize it in the presence of short-range order.

By using angle resolved photoemission spectroscopy together with our simulations using amorphous Hamiltonians to directly access the electronic states in a momentum resolved manner, we reveal that, even in the absence of long-range order, a well-defined real-space length scale is sufficient to produce dispersive band structures. Moreover, we observe for the first time a repeated Fermi surface structure of duplicated annuli, reminiscent of Brillouin zone-like repetitions.

These results (2), not only lead the way to a new understanding of electronic coherence in solids, but also open the way to the realization of novel momentum-dependent quantum phenomena such as momentum pairing and spin-orbit coupling, in a much broader class of materials than the currently studied ones, lacking long range crystalline translational symmetry.

(1) Quentin Marsal, Dániel Varjas, and Adolfo G. Grushin. PNAS 117 (48) 30260-30265. 2020.
(2) Samuel T. Ciocys, Quentin Marsal et al.. arXiv:2302.05945. 2023.

Primary authors

Dr Samuel Ciocys (Lawrence Berkeley National Laboratory and UC Berkeley) Dr Quentin Marsal (Uppsala Universitet) Dr Paul Corbae (Lawrence Berkeley National Laboratory and UC Berkeley) Dr Daniel Varjas (Stockholm University) Ellis Kennedy (Lawrence Berkeley National Laboratory and UC Berkeley) Prof. Mary Scott (Lawrence Berkeley National Laboratory and UC Berkeley) Prof. Frances Hellman (Lawrence Berkeley National Laboratory and UC Berkeley) Prof. Adolfo Grushin (Institut Néel, CNRS, Université de Grenoble) Prof. Alessandra Lanzara (Lawrence Berkeley National Laboratory and UC Berkeley)

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